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Featured by the capability of multi degree-of-freedom light-field manipulations while reserving high spatial resolution, multifocal laser arrays have been widely applied in femtosecond laser micro/nanofabrication, optical trapping, etc. However, for lens diffraction, the smaller momentum spread along the optical axis with respect to that in the transverse direction could introduce a larger position spread in real space, which in turn leads to lower axial resolution than the transverse resolution. The anisotropy of the focused laser beam, inherent regardless of paraxial or tight-focusing cases, has been a great hurdle for laser printing of functional microdevices with precise control on feature size and improved mechanical performances. To this end, in this research, a feasible method for generation of isotropic focused laser beam with quasi-spherical 3D point spread function (PSF) is developed based on vectorial light field modulation. We demonstrate that through simultaneous implementation of phase modulation and amplitude modulation, homogeneous multifocal array with quasi-spherical focal spots can be generated. Particularly, with the use of a well-designed annular mask, the suppression on the axial spread of field is accomplished via accurate control on the coherent superposition of the orthogonal radially polarized beam (RPB) and azimuthally polarized beam (APB) in the focal region since the depolarized axial component of the AP beam vanishes in vicinity of the gaussian focus even under tight focusing condition. Using the proposed method, isotropic 3D PSF with identical axial and transverse FWHM of 0.71λ is achieved. Meanwhile, based on iterative phase retrieval algorithm, phase-only holograms are designed and employed transforming the incident wavelet as the summation of sub-wavelets, yielding multiple converging sites in 3D space, thereby generating the multifocal array. We further present the synthesis of quasi-spherical multifocal array. A high uniformity up to 99% for a 10-by-10 multifocal array, in which the single focus elements share near-identical axial and transverse FWHM, being 0.76λ on average. The standard deviation of the axial and transverse FWHM of the multifocal array are evaluated be 0.005λ and 0.019λ, respectively, highlighting the features of high uniformity and isotropy. The reported strategy renders precise control on the axial feature size and is potential for the application in high-precision parallel laser printing technique.
Schematic diagram of the principle of synthesizing longitudinal super-resolution quasi-spherical multifocal arrays based on the superposition principle of cylindrical vector light modulation
(a) The standard deviation of the full width at half maximum in the five directions of the composite focus under different amplitude ratios of angularly polarized beam and radially polarized beam; (b) Field strength curves of the intensity distribution of the synthetic focus along different directions; (c)~(e) Azimuthal polarized beam superimposed on radially polarized beam to generate a two-dimensional intensity distribution of the composite focus
(a)~(b) Two-dimensional light field intensity distributions of spherical foci generated by superposition in the x-z plane, as well as lateral and longitudinal dimensions at different thresholds and different objective NAs, where the dotted line is the longitudinal dimension and the solid line is the transverse dimension; (c) The ratio of the longitudinal and transverse full width at half maximum of the focal point for angularly polarized light to radially polarized light at different threshold intensities and numerical apertures
(a) Radial polarized beam multifocal array with different number of focal points; (b) The variation of uniformity and iteration number with the number of different foci
(a), (d) The x-y cross-section (g) of the quasi-spherical multifocal array obtained by focusing and stacking the modulated angularly polarized light (a) and the modulated radially polarized light (d); (b), (e) The x-z profile (h) of the quasi-spherical multifocal array obtained by focusing the modulated angularly polarized light (b) and the modulated radially polarized light (e); (c), (f), (i) are magnifications of the marked foci in (b), (e), (h), respectively
(a) The lateral light field intensity distribution at the focal point of the synthetic quasi-spherical multifocal array; (b) Comparison of the light field intensity curves of the maximum focus and the minimum focus on the x-y plane; (c) The field intensity curves of the light intensity distribution of the maximum focus and the minimum focus in the x-z plane along different directions; (d) Three-dimensional light intensity distribution of synthetic longitudinal super-resolution quasi-spherical multifocal arrays